Browsing by Author "Mokgalapa, Naphtali Malesela"
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- ItemTheoretical investigation of dielectrophoresis and electrophoresis as techniques for silver deflections(Stellenbosch : Stellenbosch University, 2012-12) Mokgalapa, Naphtali Malesela; Wyngaardt, Shaun M.; Dobson, Robert Thomas; Stellenbosch University. Faculty of Science. Dept. of Physics.ENGLISH ABSTRACT: The primary circuit components of very high temperature reactors (VHTRs) experience various unwanted fission products such as Kr, Xe, I, Cs, Sr, and Ag. These particle are generated during normal operation of the reactor from abaration, cracks and/or deffects are transported by the helium coolant. The main candidate that has been identified as a cause for concern and the focus of research to minimizing radioactive contamination of the reactor coolant circuit is silver. This is because the design of the coated particles limits the release of fission products into the coolant except for silver(Ag110m). Ag110m is a long lived metallic fission product formed inside the nuclear reactor core and is the only known element released out of the coated particles into the coolant at any temperature above 1150 ◦C when the reactor starts to heat up. The release occurs on intact coated particles, failed particles and also from defective particles. The amount of released silver is initially small and occurs as the pebble heats up and this is strongly dependent on the temperature of the core. It is therefore able to reach the surface of the reactor core and enter into the Helium coolant flowing throughout the reactor. Thus Ag110m will be circulated through the reactor circuit until it reaches the cooler sides of the main power system (MPS) where it will start to plate out. The presence of this radioactive silver in the primary circuit components may result in unwanted maintenance problems from a radiation hazard point of view. The development of a method to remove particles from the helium stream is therefore needed. In this work, two theoretical deflection models used to deflect the silver particles are proposed, namely the stochastic and the deterministic deflection models. The latter describes the deflection of microparticles in a helium medium. It uses the dielectrophoresis (DEP) technique to investigate the deflection of a silver µm moving in a helium medium with the bulk velocity of 0.021 ms−1 and subjected to a dielectrophoretic force only deflect an amount of 0.52039 nm and 4.49882 nm in the x - and z -directions on average. The former (stochastic deflection model) describes the deflection of ions and polarized particles by using probability theory, namely kinetic theory of gases. This model showed that the mean free time that the particle spends while deflected by a uniform electric field is short so much that there is not enough time for a silver particle to be appreciably deflected between collisions. For example, when an electric field of 100kV/m was applied on a single silver ion for a time of 0.1 µs, the deflection distance obtained was 33.38 mm for a free time of 0.189285 ns and under pressure and temperature conditions of 1 bar and 20◦ C. The Brownian motion was then compared to the effects of a nonuniform electric field in polarizing and deflecting an atom. This is done by comparing the Brownian motion and the polarizibility of an atom using nonuniform electric fields. It is found that the silver speed produced from Brownian motion (79.563 ms−1) is far larger than that produced from the polarizibility of an atom (4.69455×106 nms−1). The deterministic and stochastic deflection models using nonuniform electric fields proved that the dielectrophoresis technique is negligibly small in deflecting particles and cannot be used to deflect silver particles as required in a VHTR.