Masters Degrees (Physics)

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Browsing Masters Degrees (Physics) by Subject "Active systems"

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    Dynamics of an active crosslinker on a chain and aspects of the dynamics of polymer networks
    (Stellenbosch : Stellenbosch University, 2011-12) Moller, Karl; Muller-Nedebock, Kristian K.; Stellenbosch University. Faculty of Science. Dept. of Physics.
    ENGLISH ABSTRACT: Active materials are a subset of soft matter that is constantly being driven out of an equilibrium state due to the energy input from internal processes such as the hydrolysis of adenosine triphosphate (ATP) to adenosine diphosphate (ADP), as found in biological systems. Firstly, we construct and study a simple model of a flexible filament with an active crosslinker/molecular motor. We treat the system on a mesoscopic scale using a Langevin equation approach, which we analyse via a functional integral approach using the Martin-Siggia-Rose formalism. We characterise the steady state behaviour of the system up to first order in the motor force and also the autocorrelation of fluctuations of the position of the active crosslink on the filament. We find that this autocorrelation function does not depend on the motor force up to first order for the case where the crosslinker is located in the middle of the contour length of the filament. Properties that characterise the elastic response of the system are studied and found to scale with the autocorrelation of fluctuations of the active crosslink position. Secondly, we give a brief overview of the current state of dynamical polymer network theory and then propose two dynamical network models based on a Cayley-tree topology. Our first model takes a renormalisation approach and derive recurrence relations for the coupling constants of the system. The second model builds on the ideas of an Edwards type network theory where Wick’s theorem is employed to enforce the constraint conditions. Both models are examined using a functional integral approach.
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    Polymer networks with mobile force-applying crosslinks
    (Stellenbosch : University of Stellenbosch, 2011-03) Mateyisi, Mohau Jacob; Muller-Nedebock, Kristian; Boonzaaier, Leandro; University of Stellenbosch. Faculty of Science. Dept. of Physics.
    ENGLISH ABSTRACT: We construct and study a simple model for an active gel of exible polymer filaments crosslinked by a molecular motor cluster that perform reversible work while translating along the filaments. The filament end points are crosslinked to an elastic background. In this sense we employ a simplified model for motor clusters that act as slipping links that exert force while moving along the strands. Using the framework of replica theory, quenched averages are taken over the disorder which originates from permanent random crosslinking of network end points to the background. We investigate how a small motor force contributes to the elastic properties of the network. We learn that in addition to the normal elastic response for the network there is an extra contribution to the network elasticity from the motor activity. This depends on the ratio of the entropic spring constant for the linked bio-polymerchain to the spring constant of the tether of the motor.